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1 Introduction Electrocatalytic carbon dioxide reduction (CRR) to valuable chemicals is an attractive process for the recycle use of carbon dioxide , , Due to the inert chemical property of CO 2 molecular, highly efficient catalysts are necessary for electrochemical CRR Up to now, tremendous of materials have been reported with high activity, selectivity or durability as electrocatalyst. Sitcaus uacsits tsisauc istuacs austics sautics tuisacs I'm no longer definite, those are simply the letters installed specific approaches Maybe you'll see some thing from the way in which those are organized. X I' I' I' l~l~e& 4locoC.

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1 Introduction Electrocatalytic carbon dioxide reduction (CRR) to valuable chemicals is an attractive process for the recycle use of carbon dioxide , , Due to the inert chemical property of CO 2 molecular, highly efficient catalysts are necessary for electrochemical CRR Up to now, tremendous of materials have been reported with high activity, selectivity or durability as electrocatalyst. MONSIEUR LACENAIRE/ b V X l MONSIEUR LACENAIRE i b V X l j ̓t X ̃ Y j b g u h ł B f U C i ̓t X l AGarance Brocca( K X E u J) B u h 1945 N Ɍ J ꂽ t X f u V V ~ ̐l X v ɓo ꂷ \ ͎ l ł͎E l Ƃ ʈ l u X l v R ́B o } A G X A W Z t ƍ Ńj b g ̐ Y Ɍg A t @ X g R N V p ̃R b g A { } V F Ȃǐ E e n ̗L Z N g V b v I _ ܂ ޏ ̓ Y h ̐ E ɂ g b h f U C X ^ g A R N V ͐F ͍. Ci t y o f bl o o mi ng t o n dr mart i n l ut he r ki ng , j r bi rt hday ce l e brat i o n co mmi s s i o n dr m a rt i n l u t h er k i n g j r.

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Fe/N/C material is the most competitive alternative to preciousmetal catalysts for oxygen reduction In view of the present consensus on active centers, further effort is directed at maximizing the density of single Fe atoms Here, the imperfections in commonly used doping strategy of Fe for the synthesis of zeolitic imidazolateframework (ZIF)derived Fe/N/C catalysts are revealed. 16 DA Nicholson, GC Rutledge, “Molecular simulation of flowenhanced nucleation in neicosane melts under steady shear and uniaxial extension”, J Chem. Potential and solvent are explicitly included in a firstprinciples kinetic modeling of the degradation of Fe–N–C during ORR • Axial OH ligand on the metal center of Fe–N–C is unfavorable for catalysts' stability due to much increased H 2 O 2 selectivity At high potential, Fe–N–C sites may induce Fentonlike reactions to produce harmful hydroxyl radicals (•OH) from H 2 O 2.

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0 j Ë j Í ?. Fe/N/C material is the most competitive alternative to preciousmetal catalysts for oxygen reduction In view of the present consensus on active centers, further effort is directed at maximizing the density of single Fe atoms Here, the imperfections in commonly used doping strategy of Fe for the synthesis of zeolitic imidazolateframework (ZIF)derived Fe/N/C catalysts are revealed.